JP

The Emission Database for Global Atmospheric Research (EDGAR) provides a time-series of man-made emissions of greenhouse gases and short-lived atmospheric pollutants from 1970 to 2008. Mercury is included in EDGARv4.tox1, thereby enriching the spectrum of multi-pollutant sources in the database. With an average annual growth rate of 1.3% since 1970, EDGARv4 estimates that the global mercury emissions reached 1287 tonnes in 2008. Specifically, gaseous elemental mercury (GEM) (Hg0) accounted for 72% of the global total emissions, while gaseous oxidised mercury (GOM) (Hg2 +) and particle bound mercury (PBM) (Hg-P) accounted for only 22% and 6%, respectively. The less reactive form, i.e., Hg0, has a long atmospheric residence time and can be transported long distances from the emission sources. The artisanal and small-scale gold production, accounted for approximately half of the global Hg0 emissions in 2008 followed by combustion (29%), cement production (12%) and other metal industry (10%). Given the local-scale impacts of mercury, special attention was given to the spatial distribution showing the emission hot-spots on gridded 0.1° × 0.1° resolution maps using detailed proxy data. The comprehensive ex-post analysis of the mitigation of mercury emissions by end-of-pipe abatement measures in the power generation sector and technology changes in the chlor-alkali industry over four decades indicates reductions of 46% and 93%, respectively. Combined, the improved technologies and mitigation measures in these sectors accounted for 401.7 tonnes of avoided mercury emissions in 2008. A comparison shows that EDGARv4 anthropogenic emissions are nearly equivalent to the lower estimates of the United Nations Environment Programme (UNEP)'s mercury emissions inventory for 2005 for most sectors. An evaluation of the EDGARv4 global mercury emission inventory, including mercury speciation, was performed using the GEOS-Chem global 3-D mercury model. The model can generally reproduce both spatial variations and long-term trends in total gaseous mercury concentrations and wet deposition fluxes.

 

© 2014 the authors

Water availability is a growing concern globally (UN, 2012). Many countries are affected by water scarcity and quality issues (Postel, 2000). The United States (U.S.) is no exception, with the Colorado and the Rio Grande rivers so severely exploited that they often do not reach the oceans. The exploitation of U.S. water resources is the consequence of growing population and economic activity, and lack of conservation measures. Under the threat of climate change and consequently a change in water resources, water issues are even more pressing. To investigate the issue of water allocation and scarcity for the U.S., we use a computable general equilibrium (CGE) model to drive water requirements in an integrated assessment framework. Specifically, we apply a specially tailored version of the Integrated Global System Model – Water Resource System (IGSM-WRS) model (Strzepek et al., 2012), which draws on the water system module (WSM) developed by the International Food Policy Research Institute (Rosegrant et al. 2008). WRS allows the linkage of WSM with the IGSM (Sokolov et al. 2005). This integrated assessment framework facilitates evaluation of both the direct (via a geophysical model) and indirect (thanks to a CGE model) impacts of climate policy on water scarcity. Taking advantage of data available for the U.S., we model water at a 99-basin level (instead of the 14 regions in the global WRS model). Detailed economic inputs are supplied by the 11-region U.S. Regional Economic Policy (USREP) model (Rausch et al. 2009). This CGE model also provides detailed energy demand which allows a better estimation of water requirements for mining and thermoelectric power generation.

The Probabilistic Collocation Method (PCM) has been proven to be an efficient general method of uncertainty analysis in atmospheric models (Tatang et al 1997, Cohen&Prinn 2011). However, its application has been mainly limited to urban- and regional-scale models and chemical source-sink models, because of the drastic increase in computational cost when the dimension of uncertain parameters increases. Moreover, the high-dimensional output of global models has to be reduced to allow a computationally reasonable number of polynomials to be generated. This dimensional reduction has been mainly achieved by grouping the model grids into a few regions based on prior knowledge and expectations; urban versus rural for instance. As the model output is used to estimate the coefficients of the polynomial chaos expansion (PCE), the arbitrariness in the regional aggregation can generate problems in estimating uncertainties. To address these issues in a complex model, we apply the probabilistic collocation method of uncertainty analysis to the aerosol representation in MOZART-4, which is a 3D global chemical transport model (Emmons et al., 2010). Thereafter, we deterministically delineate the model output surface into regions of homogeneous response using the method of Principal Component Analysis. This allows the quantification of the uncertainty associated with the dimensional reduction. Because only a bulk mass is calculated online in Mozart-4, a lognormal number distribution is assumed with a priori fixed scale and location parameters, to calculate the surface area for heterogeneous reactions involving tropospheric oxidants. We have applied the PCM to the six parameters of the lognormal number distributions of Black Carbon, Organic Carbon and Sulfate. We have carried out a Monte-Carlo sampling from the probability density functions of the six uncertain parameters, using the reduced PCE model. The global mean concentration of major tropospheric oxidants did not show a significant variation in response to the variation in input parameters. However, a substantial variation at regional and temporal scale has been found. Tatang M. A., Pan W., Prinn R G., McRae G. J., An efficient method for parametric uncertainty analysis of numerical geophysical models, J. Gephys. Res., 102, 21925-21932, 1997. Cohen, J.B., and R.G. Prinn, Development of a fast, urban chemistry metamodel for inclusion in global models,Atmos. Chem. Phys., 11, 7629-7656, doi:10.5194/acp-11-7629-2011, 2011. Emmons L. K., Walters S., Hess P. G., Lamarque J. -F., P_ster G. G., Fillmore D., Granier C., Guenther A., Kinnison D., Laepple T., Orlando J., Tie X., Tyndall G., Wiedinmyer C., Baughcum S. L., Kloster J. S., Description and evaluation of the Model for Ozone and Related chemical Tracers, version 4 (MOZART-4). Geosci. Model Dev., 3, 4367, 2010.

This study aims to assess how high-latitude vegetation may respond under various climate scenarios during the 21st century with a focus on analyzing model parameters induced uncertainty and how this uncertainty compares to the uncertainty induced by various climates. The analysis was based on a set of 10,000 Monte Carlo ensemble Lund-Potsdam-Jena (LPJ) simulations for the northern high latitudes (45oN and polewards) for the period 1900–2100. The LPJ Dynamic Global Vegetation Model (LPJ-DGVM) was run under contemporary and future climates from four Special Report Emission Scenarios (SRES), A1FI, A2, B1, and B2, based on the Hadley Centre General Circulation Model (GCM), and six climate scenarios, X901M, X902L, X903H, X904M, X905L, and X906H from the Integrated Global System Model (IGSM) at the Massachusetts Institute of Technology (MIT). In the current dynamic vegetation model, some parameters are more important than others in determining the vegetation distribution. Parameters that control plant carbon uptake and light-use efficiency have the predominant influence on the vegetation distribution of both woody and herbaceous plant functional types. The relative importance of different parameters varies temporally and spatially and is influenced by climate inputs. In addition to climate, these parameters play an important role in determining the vegetation distribution in the region. The parameter-based uncertainties contribute most to the total uncertainty. The current warming conditions lead to a complexity of vegetation responses in the region. Temperate trees will be more sensitive to climate variability, compared with boreal forest trees and C3 perennial grasses. This sensitivity would result in a unanimous northward greenness migration due to anomalous warming in the northern high latitudes. Temporally, boreal needleleaved evergreen plants are projected to decline considerably, and a large portion of C3 perennial grass is projected to disappear by the end of the 21st century. In contrast, the area of temperate trees would increase, especially under the most extreme A1FI scenario. As the warming continues, the northward greenness expansion in the Arctic region could continue.

© 2012 The Authors

We examine the sensitivity of the biogeography of nitrogen fixers to a warming climate and increased aeolian iron deposition in the context of a global earth system model. We employ concepts from the resource-ratio theory to provide a simplifying and transparent interpretation of the results. First we demonstrate that a set of clearly defined, easily diagnosed provinces are consistent with the theory. Using this framework we show that the regions most vulnerable to province shifts and changes in diazotroph biogeography are the equatorial and South Pacific, and central Atlantic. Warmer and dustier climates favor diazotrophs due to an increase in the ratio of supply rate of iron to fixed nitrogen. We suggest that the emergent provinces could be a standard diagnostic for global change models, allowing for rapid and transparent interpretation and comparison of model predictions and the underlying mechanisms. The analysis suggests that monitoring of real world province boundaries, indicated by transitions in surface nutrient concentrations, would provide a clear and easily interpreted indicator of ongoing global change.

© 2014 the authors.

Transient eddies in the extratropical storm tracks are a primary mechanism for the transport of momentum, energy, and water in the atmosphere, and as such are a major component of the climate system. Changes in the extratropical storm tracks under global warming would impact these transports, the ocean circulation and carbon cycle, and society through changing weather patterns. I show that the southern storm track intensifies in the multimodel mean of simulations of 21st century climate change, and that the seasonal cycle of storm-track intensity increases in amplitude in both hemispheres. I use observations of the present-day seasonal cycle to confirm the relationship between storm-track intensity and the mean available potential energy of the atmosphere, and show how this quantitative relationship can be used to account for much of the varied response in storm-track intensity to global warming, including substantially different responses in simulations with different climate models. The results suggest that storm-track intensity is not related in a simple way to global-mean surface temperature, so that, for example, a stronger southern storm track in response to present-day global warming does not imply it was also stronger in hothouse climates of the past.

© 2010 National Academy of Sciences

Historically, electricity consumption has been largely insensitive to short term spot market conditions, requiring the equating of supply and demand to occur almost exclusively through changes in production. Large scale entry of demand response, however, is rapidly changing this paradigm in the electricity market located in the mid-Atlantic region of the US, called PJM. Greater demand side participation in electricity markets is often considered a low cost alternative to generation and an important step towards decreasing the price volatility driven by inelastic demand. Recent experience in PJM, however, indicates that demand response in the form of a peaking product has the potential to increase energy price level and volatility.

Currently, emergency demand response comprises the vast majority of demand side participation in PJM. This is a peaking product dispatched infrequently and only during periods of scarcity when thermal capacity is exhausted. While emergency demand response serves as a cheaper form of peaking resource than gas turbines, it has recently contributed to increases in energy price volatility by setting price at the $1,800/MWh price cap, substantially higher than the marginal cost of most thermal generation. Additionally, the entry of demand response into the PJM capacity market is one of primary drivers for capacity prices declining by over fifty percent. This study investigates the large penetration of emergency demand response in PJM and the implications for the balance between energy and capacity prices and energy price volatility. A novel model is developed that dynamically simulates generation entry and exit over a long term horizon based on endogenously determined energy and capacity prices. The study finds that, while demand response leads to slight reductions in total generation cost, it shifts the bulk of capacity market revenues into the energy market and also vastly increases energy price volatility.

This transition towards an energy only market will send more accurate price signals to consumers as costs are moved out of the crudely assessed capacity charge and into the dynamic energy price. However, the greater volatility will also increase the risk faced by many market participants. The new market paradigm created by demand response will require regulators to balance the importance of sending accurate price signals to consumers against creating market conditions that decrease risk and foster investment.

Land can be used in several ways to mitigate climate change, but especially under changing environmental conditions there may be implications for food prices. Using an integrated global system model, we explore the roles that these land-use options can play in a global mitigation strategy to stabilize Earth’s average temperature within 2oC of the pre-industrial level, and their impacts on agriculture. We show that an ambitious global Energy-Only climate policy that includes biofuels would likely not achieve the 2°C target. A thought-experiment where the world ideally prices land carbon fluxes combined with biofuels (Energy+Land policy) gets the world much closer. Land could become a large net carbon sink of about 178 Pg C over the 21st century with price incentives in the Energy+Land scenario. With land carbon pricing but without biofuels (a No-Biofuel scenario) the carbon sink is nearly identical to the case with biofuels but emissions from energy are somewhat higher, thereby avoiding less warming. Absent such incentives, land is either a much smaller net carbon sink (+37 Pg C – Energy-Only policy) or a net source (-21 Pg C – No-Policy). The significant tradeoff with this integrated land-use approach is that prices for agricultural products rise substantially because of mitigation costs borne by the sector and higher land prices. Share of income spent on food for wealthier regions continues to fall, but for the poorest regions, higher food prices lead to a rising share of income spent on food.

© ACS Publications

The possibility of using electricity dispatching strategies to achieve a 50% nitrogen oxide (NOx) emission reduction from electricity generating units was examined using the grid of the Electricity Reliability Council of Texas as a case study. Simulations of a hypothetical policy demonstrate that imposing higher NOx prices induces a switch from some coal-fired generation to natural gas generation, lowering NOx emissions. The simulation is for a day with relatively high electricity demand and accounts for transmission constraints. In addition to the lowering of the NOx emissions, there are co-benefits of the redispatching of generation from coal to natural gas, including reductions in the emissions of sulfur oxides (24%–71%), Hg (16%–82%) and CO2 (8.8%–22%). Water consumption was also decreased, by 4.4%–8.7%. Substantial reductions of NOx emissions can be achieved for an increased generation cost of 4–13%, which is due to the higher fuel price of gas relative to coal (assuming a price of $3.87 per MMBTU (MMBTU: million British thermal units) for natural gas, and $1.89 per MMBTU for coal). However, once the system has reduced NOx emissions by approximately 50%, there is little incremental reduction in emissions due to further increases in NOx prices.

© 2011 IOP Publishing Ltd

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